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Portishead because they're really good and wont sound to alien for your first venture. BOC just because I think you would like them alot. Try Four Tet, M83 and Venetian Snares, too (they arnt similar in any way).
oh and lets not forget Autechre's Tri Repetae++. give it a good listen and it will be your gateway.
I asked the same question a few months back and the best starters for me were:
Aphex Twin - I Care Because You Do Aphex Twin - Come To Daddy Portishead - Dummy Squarepusher - Go Plastic! Boards Of Canada - Music Has The Right To Children
I enjoyed all of them although the first listen of the Aphex Twin albums was an experience I won't forget.
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How can he see he's got flies in his eyes if he's got flies in his eyes?
my starter was Confield from Autechre. many of times i mention this, but if it wasn't for that album im not sure that i would have plunged into this music.